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Research Spending & Results

Award Detail

Awardee:TRUSTEES OF THE UNIVERSITY OF PENNSYLVANIA, THE
Doing Business As Name:University of Pennsylvania
PD/PI:
  • Arjun G Yodh
  • (215) 898-6354
  • yodh@dept.physics.upenn.edu
Award Date:09/26/2005
Estimated Total Award Amount: $ 18,000,000
Funds Obligated to Date: $ 21,669,000
  • FY 2009=$5,613,603
  • FY 2007=$3,600,000
  • FY 2008=$3,600,000
  • FY 2005=$3,600,000
  • FY 2006=$3,639,000
  • FY 2010=$1,616,397
Start Date:10/01/2005
End Date:09/30/2012
Transaction Type: Cooperative Agreements
Agency:NSF
Awarding Agency Code:4900
Funding Agency Code:4900
CFDA Number:47.049
Primary Program Source:040100 NSF RESEARCH & RELATED ACTIVIT
Award Title or Description:MRSEC: Materials Research Science and Engineering Center
Federal Award ID Number:0520020
DUNS ID:042250712
Parent DUNS ID:042250712
Program:MATERIALS RSCH SCI & ENG CENT

Awardee Location

Street:Research Services
City:Philadelphia
State:PA
ZIP:19104-6205
County:Philadelphia
Country:US
Awardee Cong. District:03

Primary Place of Performance

Organization Name:University of Pennsylvania
Street:Research Services
City:Philadelphia
State:PA
ZIP:19104-6205
County:Philadelphia
Country:US
Cong. District:03

Abstract at Time of Award

The University of Pennsylvania Materials Research Science & Engineering Center (MRSEC) will build on past success and embrace new faculty to pursue a program to integrate the design, synthesis, characterization, theory & modeling of materials. These materials range from hybrid macro-molecules and de novo proteins, with architectures & functions inspired by nature, to nano- and micro-structured hard & soft materials with unique properties. Potential practical outcomes are in the areas of drug delivery, energy transduction, electronics, sensors, and cellular probes. The MRSEC research is organized around five Interdisciplinary Research Groups (IRGs), which target new advanced materials with potential for high-technology applications in diverse areas such as energy transduction, electronics, sensors, & cellular probes. Materials interfaces are a recurrent theme, as is the interplay between biological & synthetic constructs and composites of hard & soft materials. The MRSEC sustains an array of education and human resources development programs, whose impact will range from K-12 students and their teachers to undergraduates and faculty at minority serving institutions. It is associated with the University of Puerto Rico at Humacao through a Partnership for Research and Education in Materials (PREM). The MRSEC manages extensive shared facilities that benefit the broader research community. The MRSEC is linked with Penn's Center for Technology Transfer to license its discoveries and inventions for translational research thereby ensuring the coupling of MRSEC research to the needs of society. The MRSEC contains the following IRGs: Filamentous Networks and Structured Gels, IRG-1 explores the properties of filamentous networks with a goal to design & synthesize responsive network materials. Functional Cylindrical Assemblies, IRG-2 will synthesize semi-flexible, functional cylinders, composed of dendrimer-based polymers & self-assembling block copolymers. Synthetic Programmable Membranes, IRG-3 draws expertise from four departments to design fully integrated functional analogues of cellular membranes. De Novo Synthetic Protein Modules for Light-Capture & Catalysis, IRG-4 draws on the rich biological resource of atomic-level structures and functional mechanisms to guide design & synthesis of novel proteins as modular nano-scale materials. Oxide-based Hierarchical Interfacial Materials, IRG-5 will harness expertise in theory, synthesis, & experiment, from four departments to create and understand novel hierarchical interfacial oxide materials. Participants in the Center currently include 38 senior investigators, 12 postdoctoral associates, and 22 graduate students from seven departments. Professor Michael L. Klein directs the MRSEC.

Publications Produced as a Result of this Research

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Kuroda, K.;DeGrado, W.F.; "es as antimicrobial agents" J. Am. Chem. Soc., v.127, 2005, p.4128-4129.

Latka, A.;Han, Y.;Alsayed, A.M.;Schofield, A.B.;Yodh, A.G;Habdas, P.; "Particle dynamics in colloidal suspensions above and below the glass-liquid re-entrance transition" Europhys. Lett., v.86, 2009, p.58001.

Lau, A.W.C.;Lubensky, T.C.; "Fluctuating hydrodynamics and microrheology of a dilute suspension of swimming bacteria" Phys. Rev. E, v.80, 2009, p.011917.

Lee, C.;Li, Q. Y.;Kalb, W.;Liu, X. Z.;Berger, H.;Carpick, R.W.;Hone, J.; "Frictional characteristics of atomically thin sheets" Science, v.328, 2010, p.76-80.

Lee, K.-C.;Liu, A.J.; "New proposed mechanism of actin-polymerization-driven motility" Biophys. J., v.95, 2008, p.4529-4539.

Percec, V.; Wilson, D.A.; Leowanawat, P.; Wilson, C.J.; Hughes, A.D.; Kaucher, M.S.; Hammer, D.A.; Levine, D.H.; Kim, A.J.; Bates, F.S.; Davis, K.P.; Lodge, T.P.; Klein, M.L.; DeVane, R.H.; Aquad, E.; Rosen, B. M.; Argintaru, A.O.; ; Rissanen, K., et al. "Self-assembly of Janus-dendrimers into uniform dendrimersomes and other complex architectures" Science, v.329, 2010, p.xxxx-xxxx.

Erglis, K.;Wen, Q.;Ose, V.;Zeltins, A.;Sharipo, A.;Janmey, P.A.;Cebers, A.; "Dynamics of magnetotactic bacteria in a rotating magnetic field" Biophys. J., v.93, 2007, p.1402-1412.

Lee, K.C.;Liu, A.J.; "Force-velocity relation for actin-polymerization-driven motility from brownian dynamics simulations" Biophys. J., v.97, 2009, p.1295-1304.

Lee, M. H.;Prasad, V.;Lee, D.; "Microfluidic fabrication of stable nanoparticle-shelled bubbles" Langmuir, v.26, 2010, p.2227-2230.

Lee, M.;Choi, U. H.;Salas-de la Cruz, D.;Mittal, A.;ey, K. I.;Colby, R. H.;Gibson, H. W.; "Imidazolium polyesters: Structure-property relationships in thermal behavior, ionic conductivity, and morphology" Adv. Funct. Mater., v.21, 2011, p.708-717.

Lee, M.H.;Lee, D.; "Elastic instability of polymer-shelled bubbles formed from air-in-oil-in-water compound bubbles" Soft Matter, v.6, 2010, p.4326-4330.

Lee, M.H.;Prasad, V.;Lee, D.; "Microfluidic-based generation of fabrication of microbubbles for imaging and therapy" Patent Disclosure, v., 2010, p..

Wilson, D.A.;Wilson, C.J.;Moldoveanu, C.;Resmerita, A.M.;Corcoran, P.;Hoang, L.M.;Rosen, B.M.;Percec, V.; "Neopentylglycolborylation of aryl mesylates and tosylates catalyzed by Ni-based mixed-ligand systems activated with Zn" J. Am. Chem. Soc., v.132, 2010, p.1800-1801.

Gonella, G.;Dai, H. L.;Fry, H. C.;Therien, M. J.;Krishnan, V.;Tronin, A.;Blasie, J. K.; "Control of the orientational order and nonlinear optical response of the "push-pull" chromophore RuPZn via specific incorporation into densely packed monolayer ensembles of an amphiphilic 4-helix bundle peptide: Second harmonic generation at high c et al." J. Am. Chem. Soc., v.132, 2010, p.9693-9700.

Xu, C.;Ohno, K.;Ladmiral, V.;Milkie, D.E.;Kikkawa, J.M.;Composto, R.J.; "Simultaneous Block Copolymer and Magnetic Nanoparticle Assembly in Nanocomposite Films" Macromolecules, v.42, 2009, p.1219-1228.

Percec, V.;Imam, M.R.;Peterca, M.;Cho, W. D.;Heiney, P.A; "Self-assembling dendronized dendrimers" Israel J. Chem., v.49, 2009, p.55-70.

Percec, V.;Imam, M.R.;Peterca, M.;Wilson, D.A.;Heiney, P.A.; "Self-assembly of dendritic crowns into chiral supramolecular spheres" J. Am. Chem. Soc., v.131, 2009, p.1294-1304.

Esposito, C.;Tian, A.;Melamed, S.;Johnson, C.;Tee, S.Y.;Baumgart, T.; "Flicker spectroscopy of thermal lipid bilayer domain boundary fluctuations" Biophys. J., v.93, 2007, p.3169-3181.

Fadeev, A. Y.;DeGrado, W. F.; "Lipid membranes supported on optically transparent nanosilicas: Synthesis and application in characterization of protein-membrane interactions" J. Colloid Interface Sci., v.355, 2011, p.265-268.

Percec, V.;Peterca, M.;Tsuda, Y.;Rosen, B.M.;Uchida, S.;Imam, M.R.;Ungar, G.;Heiney, P.A; "Elucidating the structure of the Pm3n cubic phase of supramolecular dendrimers through the modification of their aliphatic to aromatic volume ratio" Chemistry (Weinheim an der Bergstrasse, Germany), v.15, 2009, p.8994-9004.

Fafarman, A. T.;Koh, W. K.;Diroll, B. T.;Kim, D. K.;Ko, D. K.;Oh, S. J.;Ye, X. C.;Doan-Nguyen, V.;Crump, M. R.;Reifsnyder, D. C.;Murray, C. B.;Kagan, C. R.; "in nanocrystal solids" J. Am. Chem. Soc., v.133, 2011, p.15753-157.

Discher, B. M.;Noy, D.;Strzalka, J.;Ye, S. X.;Moser, C. C.;Lear, J. D.;Blasie, J. K.;Dutton, P. L.; "Design of amphiphilic protein maquettes: Controlling assembly, membrane insertion, and cofactor interactions" Biochem., v.44, 2005, p.12329-123.

Discher, B.;Discher, D.;Hammer, D.; "Polymersomes and related encapsulating membranes; Issued US # 7,217,427 (5/15/2007)." Issued US # 7,217,427, v., 2007, p..

Percec, V.;Sienkowska, M.J.; "4 C by SET-DTLRP initiated from a tetrafunctional initiator" J. Polymer Sci., Part A, Polymer Chem., v.47, 2009, p.628-634.

Cerda, J.F.;Koder, R.L.;Lichtenstein, B.R.;Moser, C. M.;Miller, A.F.;Dutton, P.L.; "Hydrogen bond-free flavin redox properties: managing flavins in extreme aprotic solvents" Org. Biomol. Chem., v.6, 2008, p.2204-2212.

, T. V.;Wu, S. P.;Therien, M. J.; "Ethyne-bridged (porphinato)zinc(II)-(porphinato)iron(III) complexes: Phenomenological dependence of excited-state dynamics upon (porphinato) iron electronic structure" J. Am. Chem. Soc., v.128, 2006, p.10423-104.

Qi, T.;Grinberg, I.;Rappe, A.M.; "First-principles investigation of the highly tetragonal ferroelectric material Bi ( Zn1/2 Ti1/2 ) O3" Phys. Rev. B., v.79, 2009, p.094114.

Faiella, M.;Andreozzi, C.;de Rosales, R.T.M.;Pavone, V.;Maglio, O.;Nastri, F.;DeGrado, W.F.;Lombardi, A.; "An artificial di-iron oxo-protein with phenol oxidase activity" Nature Chemical Biology, v.5, 2009, p.882-884.

Fairfield, J. A.;Dadosh, T.;Drndic, M.; "Characterization of memory and measurement history in photoconductivity of nanocrystal arrays" Applied Physics Letters, v.97, 2010, p..

Bissonnette, M.L.Z.;Donald, J.E.;DeGrado, W.F.;Jardetzky, T.S.;Lamb, R.A.; "Functional analysis of the transmembrane domain in paramyxovirus F protein-mediated membrane fusion" J. Molecular Biol., v.386, 2009, p.14-36.

Goodman, C.M.;Choi, S.;Shandler, S.;DeGrado, W.F.; "Foldamers as versatile frameworks for the design and evolution of function" Nat. Chem. Biol., v.3, 2007, p.252-262.

Xu, N.;Haxton, T.K.;Liu, A.J.;Nagel, S.R.; "Equivalence of glass transition and colloidal glass transition in the hard-sphere limit" Phys. Rev. Lett., v.103, 2009, p..

Gopinathan, A.;Lee, K.C.;Schwarz, J.M.;Liu, A.J.; "Branching, capping, and severing in dynamic actin structures" Phys. Rev. Lett., v.99, 2007, p.058103.

Gorte, R.;Vohs, J.; "Porous electrode, solid oxide fuel cell, and method of producing the same. Issued US #6,958,196 (10/25/2005)." Issued US #6,958,196, v., 2005, p..

Xu, Y.;Zhu, X.;Yang, S.; "Crack-Free 3D Hybrid Microstructures from Photosensitive Organosilicates as Versatile Photonic Templates" ACS Nano, v.3, 2009, p.3251-3259.

Gorte, R.;Vohs, J.; "Method for solid oxide fuel cell anode preparation; Issued US #7,014,942 (3/21/2006)." Issued US #7,014,942, v., 2006, p..

Yu, Q.;Shan, Z.W.;Li, J.;Huang, X.X.;Xiao, L.;Sun, J.;Ma, E.; "Strong crystal size effect on deformation twinning" Nature, v.463, 2010, p.335-338.

Christian, D.A.;Garbuzenko, O.B.;Minko, T.;Discher, D.E.; "Polymer vesicles with a red cell-like surface charge: Microvascular imaging and in vivo tracking with near-infrared fluorescence" Macromol. Rapid Commun., v.31, 2010, p.135-141.

Jung, Y.;Yang, C.Y.;Lee, S. H.;Agarwal, R.; "Phase-change Ge-Sb nanowires: Synthesis, memory switching, and phase-instability" Nano Lett., v.9, 2009, p.2103-2108.

Jiang, X.;Fleischmann, S.;Nguyen, N.H.;Rosen, B.M.;Percec, V.; "Cooperative and synergistic solvent effects in SET-LRP of MA" J. Polym. Sci. Pol. Chem. Part a-Polymer Chemistry, v.47, 2009, p.5591-5605.

Grinberg, I.;Suchomel, M.R.;Davies, P.K.;Rappe, A.M.; "Predicting morphotropic phase boundary locations and transition temperatures in Pb-and Bi-based perovskite solid solutions from crystal chemical data and first-principles calculations" J. Appl. Phys., v.98, 2005, p.94111 (1-.

Butts, C A.;Swift, J.;Kang, S.G.;Di Costanzo, L.;Christianson, D.W.;Saven, J.G.;Dmochowski, I.J.; "Directing noble metal ion chemistry within a designed ferritin protein" Biochem., v.47, 2008, p.12729-127.

Gorte, R.;Vohs, J.; "Solid-state electrochemical NO.sub.x sensors; Issued US #7,220,343 (5/22/2007)." Issued US #7,220,343, v., 2007, p..

Yunker, P.;Zhang, Z.;Aptowicz, K.B.;Yodh, A.G.; "al structure in aging glasses" Phys. Rev. Lett, v.103, 2009, p.115701.

Gorte, R.;Vohs, J.; "Ceramic anodes and methods of producing the same; Issued US #7,740,772 (6/22/2010)" Issued US #7,740,772, v., 2010, p..

Zhang, B.;Jung, Y.;Chung, H.S.;Van Vugt, L.;Agarwal, R.; "Nanowire transformation by size-dependent cation exchange reactions" Nano Letters, v.10, 2010, p.149-155.

Grigoryan, Gevorg;Kim, Yong Ho;Acharya, Rudresh;Axelrod, Kevin;Jain, Rishabh M.;Willis, Lauren;Drndic, Marija;Kikkawa, James M.;DeGrado, William F.; "Computational design of virus-like protein assemblies on carbon nanotube surfaces" Science, v.332, 2011, p.1071-1076.

Zhang, Y.;Kulp, D.W.;Lear, J.D.;DeGrado, W.F.; "Experimental and computational evaluation of forces directing the association of transmembrane helices" J. Am. Chem. Soc, v.131, 2009, p.113411.

Nguyen, N.H.;Jiang, X.;Fleischmann, S.;Rosen, B.M.;Percec, V.; "The effect of ligand on the rate of propagation of Cu(0) wire catalyzed SET-LRP of MA in DMSO at 25 degrees C" J. Polym. Sci. Pol. Chem. Part a-Polymer Chemistry, v.47, 2009, p.5629-5638.

Dalhaimer, P.;Discher, D.E.;Lubensky, T.C.; "show liquid crystal elastomer behaviour, including soft-mode elasticity" Nat. Phys., v.3, 2007, p.354-360.

Kamien, R.D.;Nelson, D.R.;Santangelo, C.D.;Vitelli, V.; "Extrinsic curvature, geometric optics, and lamellar order on curved substrates" Phy. Rev. E., v.80, 2009, p.051703.

Imam, M.R.;Peterca, M.;Edlund, U.;Balagurusamy, V.S.K.;Percec, V.; "Dendronized supramolecular polymers self-assembled from dendritic ionic liquids" J. Polym. Sci. Pol. Chem., v.47, 2009, p.4165-4193.

Gledhill Jr, J.M.;Wand, A.J.; "SEnD NMR: Sensitivity enhanced n-dimensional NMR" J. Mag. Res., v.202, 2010, p.250-258.

Robbins, G.P.;Jimbo, M.;Swift, J.;Therien, M.J.;Hammer, D.A.;Dmochowski, I.J.; "Photoinitiated destruction of composite porphyrin- protein polymersomes" J. Am. Chem. Soc., v.131, 2009, p.3872-3874.

Peng, Y.;Wang, Z.;Alsayed, A.M.;Yodh, A.G.;Han, Y.; "Melting of colloidal crystal films" Phys. Rev. Lett., v.104, 2010, p.219901.

Percec, V.; "merization of vinyl halides; Issued US #7,026,420 (4/11/2006)." Issued US #7,026,420, v., 2006, p..

Percec, V.; "Bioinspired supramolecular liquid crystals" Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci., v.364, 2006, p.2709-2719.

Percec, V.; "Living radical polymerization of halogen-containing acrylic monomers and the formation of block copolymers therefrom; Issued US #7,345,127 (3/18/2008)." Issued US #7,345,127, v., 2008, p..

Percec, V.; "Living radical polymerization of scrylic monomers and the gormation of block copolymers therefrom; Issued US #7,470,762 (12/30/2008)." Issued US #7,470,762, v., 2008, p..

Percec, V.; "Amphiphilic dendritic dipeptides and their self-assembly into helical pores; Issued US #7,671,033 (3/2/2010)" Issued US #7,671,033, v., 2010, p..

Percec, V.; "Processes for the synthesis of dendritic macromolecules from conventional monomers; Issued US #7,776,971 B2 (8/17/2010)." Issued US #7,776,971 B2, v., 2010, p..

Percec, V.; Wilson, D. A.; Leowanawat, P.; Wilson, C. J.; Hughes, A. D.; Kaucher, M. S.; Hammer, D.A.; Levine, D. H.; Kim, A. J.; Bates, F. S.; Davis, K. P.; Lodge, T. P.; Klein, M.L.; DeVane, R. H.; Aqad, E.; Rosen, B. M.; Argintaru, A. O., et al. "Self-Assembly of Janus dendrimers into uniform dendrimersomes and other complex architectures" Science, v.328, 2010, p.1009-1014.

Percec, V.;Aqad, E.;Peterca, M.;Rudick, J. G.;Lemon, L.;Ronda, J. C.;De, B. B.;Heiney, P. A.;Meijer, E. W.; "Steric communication of chiral information observed in dendronized polyacetylenes" J. Am. Chem. Soc., v.128, 2006, p.16365-163.

Percec, V.;Asandei, A.; "Process for the living radical polymerization of chlorine containing monomers. US Patent 6,838,535" US Patent 6,838,535, v., 2005, p..

Percec, V.;Dulcey, A. E.;Peterca, M.;Ilies, M.;Nummelin, S.;Sienkowska, M. J.;Heiney, P. A.; "Principles of self-assembly of helical pores from dendritic dipeptides" Proc. Natl. Acad. Sci. USA, v.103, 2006, p.2518-2523.

Chen, K.;Manning, M. L.;Yunker, P. J.;Ellenbroek, W. G.;Zhang, Z. X.;Liu, A. J.;Yodh, A. G.; "Measurement of correlations between low-frequency vibrational modes and particle rearrangements in quasi-two-dimensional colloidal glasses" Phys. Rev. Lett., v.107, 2011, p.108301.

Katz, J.S.;Zhong, S.;Ricart, B.G.;Pochan, D.J.;Hammer, D.A.;Burdick, J.A.; "Modular synthesis of biodegradable diblock copolymers for designing functional polymersomes" J. Am. Chem. Soc., v.132, 2010, p.3654-3655.

Kaucher, M.S.;Peterca, M.;Dulcey, A.E.;Kim, A.J.;Vinogradov, S.A.;Hammer, D.A.;Heiney, P.A.;Percec, V.; "Selective transport of water mediated by porous dendritic dipeptides" J. Am. Chem. Soc, v.129, 2007, p.11698-116.

Khare, K.;Zhou, J.;Yang, S.; "Tunable open-channel microfluidics on soft poly(dimethylsiloxane) (PDMS) substrates with sinusoidal grooves" Langmuir, v.25, 2009, p.12794-127.

Kim, A.J.;Biancaniello, P.L.;Crocker, J.C.; "Engineering DNA-mediated colloidal crystallization" Langmuir, v.22, 2006, p.1991-2001.

Fischbein, M. D.;Drndic, M.; "Electron beam nanosculpting of suspended graphene sheets" Appl. Phys. Lett., v.93, 2008, p..

Guo, L.;Gai, F.; "Heterogeneous diffusion of a membrane-bound pHLIP peptide" Biophys. J., v.98, 2010, p.2914-2922.

Guo, L.;Park, J.H.;Lee, T.;Chowdhury, P.;Lim, M.;Gai, F.; "Probing the role of hydration in the unfolding transitions of carbonmonoxy myoglobin and apomyoglobin" J. Phys. Chem. B, v.113, 2009, p.6158-6163.

Guo, L.;Smith-Dupont, K. B.;Gai, F.; "Diffusion as a probe of peptide-induced membrane domain formation" Biochem., v.50, 2011, p.2291-2297.

Rosen, B M.;Wilson, C.J.;Wilson, D.A.;Peterca, M.;Imam, M.R.;Percec, V.; "Dendron-mediated self-assembly, disassembly, and self-organization of complex systems" Chem. Rev., v.109, 2009, p.6275-6540.

Biancaniello, P.L.;Crocker, J.C.;Hammer, D.A.;Milam, V.T.; "DNA-mediated phase behavior of microsphere suspensions" Langmuir, v.23, 2007, p.2688-2693.

Brown, A. E. X.;Discher, D.E.; "Conformational changes and signaling in cell and matrix physics" Current Biology, v.19, 2009, p.781-789.

Bell, C. B.;Calhoun, J.R.;Bobyr, E.;Wei, P.P.;Hedman, B.;Hodgson, K.O.;DeGrado, W.F.;Solomon, E.I.; "Spectroscopic definition of the biferrous and biferric sites in de novo designed four-helix bundle DFsc peptides: Implications for O (2) reactivity of binuclear non-heme iron enzymes (dagger)" Biochemistry, v., 2009, p..

Lee, S-H.;Jung, Y.;Agarwal, R.; "Size-dependent surface-induced heterogeneous nucleation driven phase-change in Ge" Nano Lett., v.8, 2008, p.3303-3309.

Legant, W.R.;Pathak, A.;Yang, M.T.;Deshpande, V.S.;McMeeking, R.M.;Chen, C.S.; "Microfabricated tissue gauges to measure and manipulate forces from 3D microtissues" Proc. Natl. Acad. Sci. USA, v.106, 2009, p.10097-101.

Lehmann, A.;Lanci, C.J.;Petty II, T.J.;Kang, S.-G.;Saven, J.G.; "Computational protein design" Protein Folding and Misfolding and Aggregation; Classical Themes and Novel Approaches. Royal Society of Chemistry, v., 2008, p.74-79.

Lehmann, A.;Saven, J. G.; "Computational design of four-helix bundle proteins that bind nonbiological cofactors" Computational design of four-helix bundle proteins that bind nonbiological cofactors, in Biotechnol. Prog. (Proceedinds of First International Conference on Biomolecular Engineering (ICBE), v.24, 2008, p.74-79.

Levental, I.;Byfield, F. J.;Chowdhury, P.;Gai, F.;Baumgart, T.;Janmey, P.A.; "Cholesterol-dependent phase separation in cell-derived giant plasma-membrane vesicles" Biochem. J., v.424, 2009, p.163-167.

Levental, I.;Cebers, A.;Janmey, P.A.; "Combined electrostatics and hydrogen bonding determine intermolecular interactions between polyphosphoinositides" J. Am. Chem. Soc., v.130, 2008, p.9025-9030.

Levental, I.;Christian, D.A.;Wang, Y. H.;Madara, J J.;Discher, D.E.;Janmey, P.A.; "Calcium-dependent lateral organization in phosphatidylinositol 4,5-bisphosphate (PIP2)- and cholesterol-containing monolayers" Biochem., v.48, 2009, p.8241-8248.

Lee, C.;Li, Q. Y.;Kalb, W.;Liu, X. Z.;Berger, H.;Carpick, R.W.;Hone, J.; "Frictional characteristics of atomically thin sheets" Science, v.328, 2010, p.76-80.

Lee, K.C.;Liu, A.J.; "Force-velocity relation for actin-polymerization-driven motility from brownian dynamics simulations" Biophys. J., v.97, 2009, p.1295-1304.

Levental, I.;Janmey, P.A.;Cebers, A.; "Electrostatic contribution to the surface pressure of charged monolayers containing polyphosphoinositides" Biophys. J., v.95, 2008, p.1199-1205.

Li, D. B.;Bonnell, D. A.; "Controlled patterning of ferroelectric domains: Fundamental concepts and applications" Ann. Rev. Mater. Res., v.38, 2008, p.351-368.

Li, D. B.;Strachan, D. R.;Ferris, J. H.;Bonnell, D. A.; "Polarization reorientation in ferroelectric lead zirconate titanate thin films with electron beams" J. Mater. Res., v.21, 2006, p.935-940.

Li, D. B.;Zhao, M. H.;Garra, J.;Kolpak, A. M.;Rappe, A. M.;Bonnell, D. A.;Vohs, J. M.; "Direct in situ determination of the polarization dependence of physisorption on ferroelectric surfaces" Nat. Mater., v.7, 2008, p.473-477.

Li, D.;Bonnell, D.A.; "Patterning ferroelectric surfaces" Ann. Rev. Mater. (Clarke, D.R., ed.), v., 2008, p..

Li, J.;Singh, U. G.;Bennett, J. W.;Page, K.;Weaver, J. C.;Zhang, J. P.;Proffen, T.;Rappe, A. M.;Scott, S.;Seshadri, R.; "BaCe" Chem. Mat., v.19, 2007, p.1418-1426.

Li, Q. Y.;Lee, C.;Carpick, R. W.;Hone, J.; "Substrate effect on thickness-dependent friction on graphene" Phys. Status Solidi B-Basic Solid State Phys., v.247, 2010, p.2909-2914.

Jakubinek, M.B.;White, M.A.;Mu, M.F.;Winey, K.I.; "sites" Appl. Phys. Lett., v.96, 2010, p.083105.

Christian, D.A.;Tian, A.;Ellenbroek, W.G.;Levental, I.;Rajagopal, K.;Janmey, P.A.;Liu, A.J.;Baumgart, T.;Discher, D.E.; "Spotted vesicles, striped micelles and Janus assemblies induced by ligand binding" Nature Materials, v.8, 2009, p.843-849.

Lichtenstein, B.R.;Cerda, J.F.;Koder, R.L.;Dutton, P.L.; "Reversible proton coupled electron transfer in a peptide-incorporated naphthoquinone amino acid" Chem. Comm., v.2009, 2009, p.168-170.

Lipski, A.M.;Jaquiery, C.;Choi, H.;Eberli, D.;Stevens, M.;Martin, I.;Chen, I.-W.;Shastri, V.P.; "Nanoscale engineering of biomaterial surfaces" Adv. Mater., v.19, 2007, p.553-557.

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Zhang, L.;Swift, J.;Butts, C.A.;Yerubandi, V.;Dmochowski, I.J.; "Structure and activity of apoferritin-stabilized gold nanoparticles" J. Inorganic Biochem., v.101, 2007, p.1719-1729.

Zhang, T. G.;Zhao, Y. X.;Song, K.;Asselberghs, I.;Persoons, A.;Clays, K.;Therien, M. J.; "Electronic modulation of hyperpolarizable (porphinato)zinc(II) chromophores featuring ethynylphenyl-, ethynylthiophenyl-, ethynylthiazolyl-, and ethynylbenzothiazolyl-based electron-donating and -accepting moieties" Inorg. Chem., v.45, 2006, p.9703-9712.

Zhang, Y.;Kulp, D.W.;Lear, J.D.;DeGrado, W.F.; "Experimental and computational evaluation of forces directing the association of transmembrane helices" J. Am. Chem. Soc, v.131, 2009, p.113411.

Zhang, Y.;Matsumoto, E. A.;Peter, A.;Lin, P.C.;Kamien, R.D.;Yang, S.; "scale assembly of complex structures via harnessing of elastic instability" Nano Letters, v.8, 2008, p.1192-1196.

Zhang, Y.;Reed, J.C.;Yang, S.; "Creating a library of complex metallic nanostructures via harnessing pattern transformation of a single PDMS membrane" ACS Nano, v.3, 2009, p.*Cover 24.

Zhang, Z.;Xu, N.;Chen, D.T.N.;Yunker, P.;Alsayed, A. M.;Aptowicz, K.B.;Habdas, P.;Liu, A.J.;Nagel, S.R.;Yodh, A.G.; "Thermal vestige of the zero-temperature jamming transition" Nature, v.459, 2009, p.230-233.

Chandra, D.;Yang, S.; "Capillary-force-Induced clustering of micropillar arrays: Is it caused by isolated capillary bridges or by the lateral capillary meniscus interaction force?" Langmuir, v.25, 2009, p.10430-104.

Zhao, M.H.;Bonnell, D.A.;Vohs, J.M.; "Effect of ferroelectric polarization on the adsorption and reaction of ethanol on BaTiO3" Surf. Sci., v.602, 2008, p.2849-2855.

Zhao, M.H.;Bonnell, D.A.;Vohs, J.M.; "Influence of ferroelectric polarization on the energetics of the reaction of 2-fluoroethanol on BaTiO" Surface Science, v.603, 2009, p.284-290.

Zhao, M.S.H.;Bonnell, D.A.;Vohs, J.M.; "Ferroelectric polarization dependent interactions at Pd-LiNbO3(0001) interfaces" J. Vac. Sci. Technol. A, v.27, 2009, p.1337-1342.

Zhou, N. C.;Xu, C.;Burghardt, W. R.;Composto, R.J.;Winey, K I.; "Phase behavior of polystyrene and poly (styrene-ran-styrene sulfonate) blends" Macromolecules, v.39, 2006, p.2373-2379.

Zhou, N.C.;Chan, C.D.;Winey, K.I.; "Reconciling STEM and X-ray scattering data to determine the nanoscale ionic aggregate morphology in sulfonated polystyrene ionomers" Macromolecules, v.41, 2008, p.6134-6140.

Zhu, T.;Li, J.; "Ultra-strength materials" Prog. Mater. Sci., v.55, 2010, p.710-757.

Zhu, X.;Zhang, Y.;Chandra, D.;Cheng, S.-C.;Kikkawa, J.M.;Yang, S.; "Two-dimensional photonic crystals with anisotropic unit cells imprinted from PDMS membranes under elastic deformation" Photonic and Phononic Crystal Materials and Devices IX http://link.aip.org/link/?PSI/7223/72231C/1, v.7223, 2009, p.72231C-6.

Zhu, X.L.;Zhang, Y.;Chandra, D.;Cheng, S.C.;Kikkawa, J.M.;Yang, S.; "Two-dimensional photonic crystals with anisotropic unit cells imprinted from poly(dimethylsiloxane) membranes under elastic deformation" Appl. Phys. Lett., v.93, 2008, p.911.

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Zou, H. L.;Therien, M.J.;Blasie, J.K.; "Structure and dynamics of an extended conjugated NLO chromophore within an amphiphilic 4-helix bundle peptide by molecular dynamics simulation" J. Phys. Chem. B, v.112, 2008, p.1350-1357.

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Moser, C.C.;Oxyczka, A.;Dutton, P.L.; "Short-circuit proofing Mitchell" Photosynthesis: Fundamental Aspects to Global Perspectives, v., 2005, p.pp. 427-4.

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Johnson, R.R.;Rego, B.J.;Johnson, A.T.C.;Klein, M.L.; "Computational study of a nanobiosensor: A single-walled carbon nanotube functionalized with the coxsackie-adenovirus receptor" J. Phys. Chem. B, v.113, 2009, p.11589-115.

Bonnell, D.A.;Garra, J.; "Scanning probe microscopy of oxide surfaces: atomic structure and properties" Rep. Prog. Phys., v.71, 2008, p.044501.

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Kraya, R.;Kraya, L. Y.;Bonnell, D.A.; "Orientation controlled Schottky barrier formation at Au nanoparticle-SrTiO" Nano Lett., v.10, 2010, p.1224-1228.

Krishnan, V.;Tronin, A.;Strzalka, J.;Fry, H. C.;Therien, M.J.;Blasie, J.K.; "Control of the orientational order and nonlinear optical response of the "Push-Pull" chromophore RuPZn via specific incorporation into densely packed monolayer ensembles of an amphiphilic four-helix bundle peptide: characterization of the peptide-c et al." J. Am. Chem. Soc., v.132, 2010, p.11083-110.

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Park, S.;Xu, Y.;Stowell, X. F.;Gai, F.;Saven, J. G.;Boder, E. T.; "Limitations of yeast surface display in engineering proteins of high thermostability" Protein Engineering Design and Selection, v.19, 2006, p.211-217.

Elabd, Y. A.;Napadensky, E.;Walker, C.W.;Winey, K.I.; "Transport properties of sulfonated poly (styrene-b-isobutylene-b-styrene) triblock copolymers at high ion-exchange capacities" Macromolecules, v.39, 2006, p.399-407.

Jones, A.K.;Lichtenstein, B.R.;Dutta, A.;Gordon, G.;Dutton, P.L.; "Synthetic hydrogenases: Incorporation of an iron carbonyl thiolate into a designed peptide" J. Am. Chem. Soc., v.129, 2007, p.14844-+.

Ju, Y.E.;Janmey, P.A.;McCormick, M.E.;Sawyer, E.S.;Flanagan, L.A.; "Enhanced neurite growth from mammalian neurons in three-dimensional salmon fibrin gels" Biomaterials, v.28, 2007, p.2097-2108.

Jung, Y. W.;Nam, S. W.;Agarwal, R.; "on electron microscopy study of electrically-driven reversible phase change in Ge" Nano Lett., v.11, 2011, p.1364-1368.

Jung, Y.;Agarwal, R.;Yang, C. Y.; "Chalcogenide phase-change memory nanotubes for lower writing current operation" Nanotechnology, v.22, 2011, p.254012.

Wang, Z.;Alsayed, A.M.;Yodh, A.G.;Han, Y.; "Two-dimensional freezing criteria for crystallizing colloidal monolayers" J. Chem. Phys., v.132, 2010, p.154501.

Gledhill, Jr. J.M.;Walters, B.T.;Wand, A.J.; "AMORE-HX: a multidimensional optimization of radial enhanced NMR-sampled hydrogen exchange" J. Biomolecular NMR, v.45, 2009, p.233-239.

Williams, S.R.;Salas-de la Cruz, D.;Winey, K.I.;Long, T.E.; "Ionene segmented block copolymers containing imidazolium cations: Structure-property relationships as a function of hard segment content" Polymer, v.51, 2010, p.1252-1257.

Benetatos, N.M.;Chan, C.D.;Winey, K I.; "Quantitative morphology study of Cu-neutralized poly(styrene-ran-methacrylic acid) ionomers: STEM imaging, X-ray scattering, and real-space structural modeling" Macromolecules, v.40, 2007, p.1081-1088.

Jung, Y.;Lee, S-H.;Jennings, A.T.;Agarwal, R.; "Coreâ??shell heterostructured phase change nanowire multistate memory" Nano Lett., v.8, 2008, p.2056-2062.

Jung, Y.;Yang, C.Y.;Lee, S. H.;Agarwal, R.; "Phase-change Ge-Sb nanowires: Synthesis, memory switching, and phase-instability" Nano Lett., v.9, 2009, p.2103-2108.

Kamat, N. P.;Katz, J. S.;Hammer, D. A.; "Engineering polymersome protocells" J. Phys. Chem. Lett., v.2, 2011, p.1612-1623.

Kamat, N. P.;Liao, Z. Z.;Moses, L. E.;Rawson, J.;Therien, M. J.;Dmochowski, I. J.;Hammer, D. A.; "Sensing membrane stress with near IR-emissive porphyrins" Proc. Natl. Acad. Sci. USA, v.108, 2011, p.13984-139.

Kamat, N.P.;Robbins, G.P.;Rawson, J.;Therien, M.J.;Dmochowski, I.J.;Hammer, D.A.; "A generalized system for photoresponsive membrane rupture in polymersomes" Adv. Funct. Mater., v.20, 2010, p.2588-2596.

Kamat, Neha P.;Lee, Myung Han;Lee, Daeyeon;Hammer, Daniel A.; "Micropipette aspiration of double emulsion-templated polymersomes" Soft Matter, v.7, 2011, p.9863-9866.

Kamien, R.D.;Nelson, D R.;Santangelo, C.D.;Vitelli, V.; "Extrinsic curvature, geometric optics, and lamellar order on curved substrates" Phys. Rev. E, v.80, 2009, p.051703.

Collings, P.J.;Dickinson, A. J.;Smith, E.C.; "Molecular aggregation and chromonic liquid crystals" Liquid Crystals, v.37, 2010, p.701-710.

Buxboim, A.;Rajagopal, K.;Brown, A. E.X.;Discher, D.E.; "How deeply cells feel: methods for thin gels" J. Phys.-Condes. Matter, v.22, 2010, p.194116.

Jannat, R.A.;Robbins, G.P.;Ricart, B.;Dembo, M.;Hammer, D.A.; "Neutrophil adhesion and chemotaxis depend on substrate mechanics" J. Phys.: Condens. Matter, v.22, 2010, p.194117.

Chen, J.;Ye, X.C.;Murray, C.B.; "Systematic electron crystallographic studies of self-assembled binary nanocrystal superlattices" ACS Nano, v.4, 2010, p.2374-2381.

Gledhill, Jr. J.M.;Walters, B.T.;Wand, A.J.; "AMORE-HX: a multidimensional optimization of radial enhanced NMR-sampled hydrogen exchange" J. Biomolecular NMR, v.45, 2009, p.233-239.

Fleischmann, S.;V.; "SET-LRP of methyl methacrylate initiated with CCl4 in the presence and absence of air" J. Polym. Sci. Part A: Polymer Chemistry, v.48, 2010, p.2243-2250.

Kamps, A.C.;Sanchez-Gaytan, B.L.;Hickey, R.J.;Clarke, N.;Fryd, M.;Park, S J.; "Nanoparticle-directed self-assembly of amphiphilic block copolymers" Langmuir, v.26, 2010, p.14345-143.

Kang, H.;Wen, Q.;Janmey, P.A.;Tang, J.X.;Conti, E.;MacKintosh, F.C.; "Nonlinear elasticity of stiff filament networks: Strain stiffening, negative normal stress, and filament alignment in fibrin gels" J. Phys. Chem. B, v.113, 2009, p.3799-3805.

Kang, S. G.;Saven, J. G.; "Computational protein design: structure, function and combinatorial diversity" Curr. Opin. Chem. Biol., v.11, 2007, p.329-334.

Kang, Y. K.;Deria, P.;Carroll, P. J.;Therien, M. J.; "Synthesis of water-soluble poly(p-phenyleneethynylene) in neat water under aerobic conditions via Suzuki-Miyaura polycondensation using a diborylethyne synthon" Org. Lett., v.10, 2008, p.1341-1344.

Faiella, M.;Andreozzi, C.;de Rosales, R.T.M.;Pavone, V.;Maglio, O.;Nastri, F.;DeGrado, W.F.;Lombardi, A.; "An artificial di-iron oxo-protein with phenol oxidase activity" Nature Chemical Biology, v.5, 2009, p.882-884.

Kang, Y. K.;Iovine, P. M.;Therien, M.l J.; "Electron transfer reactions of rigid, cofacially compressed," Coord. Chem. Rev., v.255, 2011, p.804-824.

Kang, Y.K.;Lee, O.S.;Deria, P.;Kim, S. H.;Park, T. H.;Bonnell, D.A.;Saven, J.G.;Therien, M.J.; "Helical wrapping of single-walled carbon nanotubes by water soluble poly(p-phenyleneethynylene)" Nano Lett., v.9, 2009, p.1414-1418.

Katz, J. S.;Burdick, J.A.; "Light-responsive biomaterials: development and applications" Macromol. Biosci., v.10, 2010, p.339-348.

Katz, J. S.;Levine, D.H.;Davis, K.P.;Bates, F.S.;Hammer, D.A.;Burdick, J.A.; "Membrane stabilization of biodegradable polymersomes" Langmuir, v.25, 2009, p.4429-4434.

Ellenbroek, W. G.;Wang, Y. H.;Christian, D. A.;Discher, D. E.;Janmey, P. A.;Liu, A. J.; "Divalent Cation-Dependent Formation of Electrostatic PIP2 Clusters in Lipid Monolayers" Biophysical Journal, v.101, 2011, p.2178-2184.

Peng, Y.;Wang, Z.;Alsayed, A.M.;Yodh, A.G.;Han, Y.; "Melting of colloidal crystal films" Phys. Rev. Lett., v.104, 2010, p.219901.

Chen, H.;Gwee, L.;Choi, J.-H.;Salas-de la Curz, D.;Winey, K I.;J.-H.Elabd, Y.A.; "Ionic conduction in polymerized ionic liquids and ionic liquid-polymer mixtures" Conference Proceedings, Polymeric Materials: Science and Engineering, American Chemical Society, Salt Lake City, v.100, 2009, p.696-697.

He, X. B.;Shinoda, W.;DeVane, R.;Anderson, K.L.;Klein, M.L.; "Paramaterization of a coarse-grained model for linear alkylbenzene sulfonate surfactants and molecular dynamics studies of their self-assembly in aqueous solution" Chem. Phys. Lett., v.487, 2010, p.71-76.

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Project Outcomes Report

Disclaimer

This Project Outcomes Report for the General Public is displayed verbatim as submitted by the Principal Investigator (PI) for this award. Any opinions, findings, and conclusions or recommendations expressed in this Report are those of the PI and do not necessarily reflect the views of the National Science Foundation; NSF has not approved or endorsed its content.

With critical assistance from the National Science Foundation, the University of Pennsylvania (Penn) materials community maintained an NSF Materials Research Science & Engineering Center (MRSEC, DMR 0520020) for the period from 2005-11. The Laboratory for Research on the Structure of Matter (LRSM) at the University of Pennsylvania (Penn) hosted to the MRSEC whose broad mission was to discover new materials and innovative applications through collaborative interdisciplinary research. To this end, LRSM developed infrastructure in the form of state-of-the-art characterization tools and shared facilities locally, regionally and nationally, and LRSM faculty trained a competitive and diverse science & engineering work force that is in demand by US academe, government and industry. Per education and outreach, LRSM fosters local, regional, national and international activities and partnerships with a goal to ensure that its research and education activities are harnessed for the good of society. Finally, LRSM is fully committed to all aspects of diversity, with long-range diversity goals to improve national pools of URMs, females, and disabled persons in all STEM activities.

The MRSEC provided the core funding for LRSM activities and thus sustained both the high impact research (i.e., activities of more than 40 core faculty) and an array of education and human resources development (HRD) programs.

The 2005-2011 Penn MRSEC collaboratively pursued five major research themes: Filamentous Networks & Structured Gels; Functional Cylindrical Assemblies; Synthetic Programmable Membranes; De Novo Synthetic Protein Modules for Light-Capture & Catalysis; Oxide-based Hierarchical Interfacial Materials. Among the most exciting new materials synthesized were those based on amphiphilic dendrimers. A dendrimer is a class of repeatedly branched molecule, and an amphiphilic dendrimer employs a two-sided molecule, with water liking/disliking components, as the building block. The group created a spectacular library of hundreds of amphiphilic dendrimers which then self-assembled into a plethora of supramolecular structures including vesicles, disks, twisted ribbons, and icosahedra. Another constellation of experimentalists and theorists explored how to pattern soft colloidal particles via self-assembly. Mixtures of two distinct amphiphiles were shown to form patterned cylinders (cylindrical micelles) and spheres (spherical vesicles). Such patterned arrays, on the surface of a colloid, could prove useful for drug delivery wherein patterned cell-specific macro-molecules match receptor patterns on cells.  Two projects focused on fundamental materials physics, (1) generating new insights about so-called frustrated matter that cannot develop long-range order because geometric constraints prevent its constituents from finding their lowest energy states, and (2) identifying new kinds of electrical conductors called topological insulators. A hard-matter collaborative effort spectacularly demonstrated the manipulation of adsorbate chemistry on oxide surfaces, showing how the polarity of an oxide surface can impact adsorption and layer formation of both gas species and metal atoms. A bio-inspired research program synthesized artificial protein modules based on non-biological heteropolymers, creating the first artificial protein module that binds oxygen substantially more tightly than carbon monoxide, i.e., exactly opposite its natural protein counterparts. Finally, a general procedure was developed for growing large-area (centimeter-size) binary nanocrystal superlattice films on solid substrates, and the first such films exhibited a nanocrystal-arrangement dependent magnetoresistance.

 

The 2005-11 MRSEC hosted an array of education and outreach programs that target stu...

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